吸附
联轴节(管道)
机制(生物学)
化学
氨
化学物理
氨生产
材料科学
物理化学
物理
有机化学
量子力学
复合材料
作者
Tianyi Dai,Hang Shi,Tong‐Hui Wang,Xingyou Lang,Qing Jiang
标识
DOI:10.1002/anie.202418035
摘要
With the continuous pursuing on the improvement of catalytic activity, a catalyst performed exceeding catalytic volcano plots is desired, while it is impeded by the adsorption-energy scaling relations of reaction intermediates. Numerous efforts have been focused on optimizing the initial and final intermediates to circumvent the scaling relations for an improved performance. For a step forward, simultaneously optimizing all intermediates is essential to explore the theoretical maximum of catalytic activity. Herein, we proposed a dynamic adsorption mechanism (DAM) to independently regulate the adsorption configurations of all intermediates of electrochemical nitrogen reduction reaction (NRR). To demonstrate the DAM, a multi-site NbNi
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