材料科学
复合数
沸石咪唑盐骨架
储能
碳纤维
纳米技术
双金属片
纳米颗粒
热稳定性
光电子学
化学工程
复合材料
吸附
金属有机骨架
化学
工程类
功率(物理)
物理
有机化学
冶金
量子力学
金属
作者
Xiao Chen,Jianhang Xu,Yang Li,Yan Gao,Ge Wang
出处
期刊:SusMat
[Wiley]
日期:2023-07-23
卷期号:3 (4): 510-521
被引量:19
摘要
Abstract In response to global energy scarcity, frontiers in multifunctional composite phase change materials (PCMs) with photo‐/electro‐/magnetothermal triggers show great potential in multiple energy utilization. However, most available composite PCM candidates are inadequate for multiple energy storage applications simultaneously. Herein, a green synthetic route is proposed to develop bimetallic zeolitic imidazolate framework (ZIF)‐derived 1D–2D bridged array carbon‐based composite PCMs for simultaneous photo‐/electro‐/magnetothermal energy storage applications. As graphitization‐induced catalyst, Co nanoparticles greatly boost the formation of ZIF‐derived 1D–2D bridged array carbon framework with high graphitization and low interface electrical/thermal resistance. Benefiting from the broadband intense photon capture, fast photon/electron/phonon transport, and surface plasma resonance effect of Co nanoparticles, the resulting composite PCMs integrate advanced photo‐, electro‐, and magnetothermal storage functions. Furthermore, composite PCMs also exhibit long‐lasting shape stability, structural stability, thermal storage stability, and photo‐/electro‐/magnetothermal storage stability after undergoing multiple heating–cooling cycles. This study is promising to accelerate the major breakthroughs of advanced multifunctional carbon‐based composite PCMs toward multiple energy utilization.
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