Bioinspired Photoluminescent “Spider Web” as Ultrafast and Ultrasensitive Airflow–Acoustic Bimodal Sensor for Human–Computer Interaction and Intelligent Recognition

Nature provides massive biomimetic design inspiration for constructing structural materials with desired performances. Spider webs can perceive vibrations generated by airflow and acoustic waves from prey and transfer the corresponding information to spiders. Herein, by mimicking the perception capability and structure of a spider web, an ultrafast and ultrasensitive airflow-acoustic bimodal sensor (HOF-TCPB@SF) is developed based on the postfunctionalization of hydrogen-bonded organic framework (HOF-TCPB) on silk film (SF) through hydrogen bonds. The "spider web-like" HOF-TCPB@SF possesses light weight and high elasticity, endowing this airflow sensor with superior properties including an ultralow detection limit (DL, 0.0076 m s