Mechanically Enhanced, Environmentally Stable, and Bioinspired Charge‐Gradient Hydrogel Membranes for Efficient Ion Gradient Power Generation and Linear Self‐Powered Sensing

with rechargeability, surpassing similar devices. Density functional theory further reveals that the energy barrier of ion transport in charge-gradient membranes is lower than that in nongradient membranes. More impressively, the device can still be applied as a linear self-powered pressure sensor for monitoring human activities after the ion gradient is completely dissipated. This study elucidates the key role of the structure and design of ion-selective membranes in the artificial gel power generation system, providing new insights into the further development and multifunctional application of flexible gel power source.