烯烃
化学
组合化学
芳基
电泳剂
区域选择性
激进的
有机化学
烷基
催化作用
作者
Efrey A. Noten,Cody Ng,Robert M. Wolesensky,Corey R. J. Stephenson
出处
期刊:Nature Chemistry
[Springer Nature]
日期:2024-01-16
卷期号:16 (4): 599-606
被引量:15
标识
DOI:10.1038/s41557-023-01404-w
摘要
Arylethylamines are popular structural elements in bioactive molecules but are often made through a linear series of synthetic steps. A modular protocol to assemble arylethylamines from alkenes in one step would represent a useful advance in discovery chemistry, though current limitations preclude a generally applicable method. In this work we disclose an aminoarylation of alkenes using aryl sulfinamide reagents as bifunctional amine and arene donors. This reaction features excellent regioselectivity and diastereoselectivity on a variety of activated and unactivated substrates. Using a weakly oxidizing photocatalyst, a nitrogen radical is generated under mild conditions and adds to an alkene to form a new C–N bond. A desulfinylative aryl migration event known as a Smiles–Truce rearrangement follows to form a new C–C bond. In this manner, arylethylamines can be rapidly assembled from abundant alkene feedstocks. Moreover, chiral information from the sulfinamide can be transferred via rearrangement to a new carbon stereocentre in the product, thus advancing the development of traceless asymmetric alkene difunctionalization. Single-step addition of an aryl ring and a protected amine across an alkene is a succinct route to valuable phenethylamine products, but existing methods suffer from limited scope. Now a family of compounds containing a sulfinamide functional group have been developed to react via electrophilic radicals to yield phenethylamines through an aryl migration with precise stereochemical control.
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