金属有机骨架
二氧化碳
电化学
块(置换群论)
还原(数学)
材料科学
二氧化碳电化学还原
金属
碳纤维
无机化学
化学
冶金
有机化学
电极
复合材料
吸附
一氧化碳
物理化学
数学
催化作用
几何学
复合数
作者
Xinyu Wu,Jianfeng Lu,Zihao Zhu,Sui‐Jun Liu,He‐Rui Wen
标识
DOI:10.1016/j.cclet.2024.110151
摘要
In recent years, reducing carbon emissions to achieve carbon neutrality has become an urgent issue for environmental protection and sustainable development. Converting CO2 into valuable chemical products through electrocatalysis powered by renewable electricity exhibits great potential. However, the electro-reduction of CO2 heavily relies on efficient catalysts to overcome the required energy barrier due to the high stability of CO2. P-block metal-based MOFs and MOF-derived catalysts have been proven to be efficient catalysts for electrochemical CO2 reduction reaction (CO2RR) due to their unique electronic structure and clear active sites. However, factors such as conductivity and stability limit the practical application of p-block metal-based MOFs and MOF-derived catalysts. In this review, we summarize the latest progress of MOFs and MOF-derived catalysts based on typical p-block metals in the field of CO2RR. Then the modification strategies for MOFs-based catalysts and the related catalytic mechanism are briefly introduced. Furthermore, we offer the challenges and prospects of p-block metal-based MOFs and MOF-derived catalysts in the hope of providing guidance for potential applications.
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