阳极
电池(电)
水溶液
锌
腐蚀
化学工程
材料科学
无机化学
极化(电化学)
电偶阳极
电化学
化学
冶金
电极
阴极保护
有机化学
物理化学
物理
功率(物理)
量子力学
工程类
作者
Kaiyong Feng,Yunyu Zhao,Ze Liu,Yingjian Yu
标识
DOI:10.1016/j.jcis.2024.08.253
摘要
Aqueous zinc-ion batteries (AZIBs) have garnered attention from researchers for their high theoretical capacity, safety, and low cost. However, the uncontrolled growth of zinc (Zn) dendrites and spontaneous corrosion reactions on the Zn anode significantly compromise the cycle life of AZIBs. This paper proposes the utilization of a novel zeolitic imidazole framework (ZIF-N) material with zincophilicity and hydrophilicity for modifying the Zn anode of AZIBs. ZIF-N incorporates numerous electron-withdrawing nitro groups at the Zn/ZIF-N interface to regulate the uneven electron distribution on the Zn anode. The modified Zn anode (Zn@ZIF-N) exhibits a lower polarization ratio (32.18 mV at 4 mA cm
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