材料科学
反射损耗
碳纳米管
纳米颗粒
化学气相沉积
复合材料
无定形碳
无定形固体
吸收(声学)
兴奋剂
衰减
复合数
化学工程
纳米技术
光电子学
光学
物理
工程类
有机化学
化学
作者
Chengjuan Wang,Yanxiang Wang,Haotian Jiang,Xiaodan Xu,Yang Yue,Bowen Cui,Mengfan Li,Zhenhao Xu
标识
DOI:10.1016/j.ceramint.2022.09.261
摘要
Highly efficient and multifunctional electromagnetic wave (EMW) absorbers which can be easily processed are desirably required. Herein, cupric ammonia is creatively adopted as the catalyst precursor of the in-situ growth of carbon nanotubes (CNTs) onto carbon fiber (CF) during chemical vapor deposition. Typically, when prepared at 750 °C, N/S co-doped bamboo-like amorphous CNTs/CF was successfully synthesized, while some Cu nanoparticles were remained in CNT forests. The sample obtains an excellent absorption toward EMWs, demonstrating a minimal reflection loss of −59.28 dB at 14.1 GHz with an ultrathin thickness of 1.42 mm. Concurrently, it is over a relatively broad effective absorption bandwidth (EAB) of 3.3 GHz (12.3–15.6 GHz) with 31% loading in the paraffin matrix. And the EAB value of CA-700 reaches 3.7 GHz (14.3–18 GHz) at merely 1.45 mm. The satisfying attenuation performance mainly originates from the synergistic effects of continuous three-dimensional conducting networks, abundant interfaces, sufficient defects, and the well impedance matching. Moreover, all as-prepared samples could be potentially used as reinforcements of resin matrix composites with high strength. Therefore, a facile route is provided to produce thin, lightweight, superior and high-strength EMW absorbing materials based on CF and CNTs.
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