Particulate matter pollution over China and the effects of control policies

微粒 质量浓度(化学) 环境科学 空气质量指数 污染 空气污染 北京 环境化学 硫酸盐 中国 硝酸盐 环境工程 化学 地理 气象学 生态学 有机化学 物理化学 考古 生物
作者
Jiandong Wang,Bin Zhao,Shuxiao Wang,Fumo Yang,Jia Xing,Lidia Morawska,Aijun Ding,Markku Kulmala,Veli‐Matti Kerminen,Joni Kujansuu,Zifa Wang,Dian Ding,Xiaoye Zhang,Huanbo Wang,Mi Tian,Tuukka Petäjä,Jingkun Jiang,Jiming Hao
出处
期刊:Science of The Total Environment [Elsevier]
卷期号:584-585: 426-447 被引量:347
标识
DOI:10.1016/j.scitotenv.2017.01.027
摘要

China is one of the regions with highest PM2.5 concentration in the world. In this study, we review the spatio-temporal distribution of PM2.5 mass concentration and components in China and the effect of control measures on PM2.5 concentrations. Annual averaged PM2.5 concentrations in Central-Eastern China reached over 100μgm-3, in some regions even over 150μgm-3. In 2013, only 4.1% of the cities attained the annual average standard of 35μgm-3. Aitken mode particles tend to dominate the total particle number concentration. Depending on the location and time of the year, new particle formation (NPF) has been observed to take place between about 10 and 60% of the days. In most locations, NPF was less frequent at high PM mass loadings. The secondary inorganic particles (i.e., sulfate, nitrate and ammonium) ranked the highest fraction among the PM2.5 species, followed by organic matters (OM), crustal species and element carbon (EC), which accounted for 6-50%, 15-51%, 5-41% and 2-12% of PM2.5, respectively. In response to serious particulate matter pollution, China has taken aggressive steps to improve air quality in the last decade. As a result, the national emissions of primary PM2.5, sulfur dioxide (SO2), and nitrogen oxides (NOX) have been decreasing since 2005, 2006, and 2011, respectively. The emission control policies implemented in the last decade could result in noticeable reduction in PM2.5 concentrations, contributing to the decreasing PM2.5 trends observed in Beijing, Shanghai, and Guangzhou. However, the control policies issued before 2010 are insufficient to improve PM2.5 air quality notably in future. An optimal mix of energy-saving and end-of-pipe control measures should be implemented, more ambitious control policies for NMVOC and NH3 should be enforced, and special control measures in winter should be applied. 40-70% emissions should be cut off to attain PM2.5 standard.
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