Dual-Sided Superhydrophobic Laser-Induced Graphene Evaporator for Efficient Desalination and Brine Treatment under High Salinity

The immense energy footprint of desalination and brine treatment is a barrier to a green economy. Interfacial evaporation (IE) offers a sustainable approach to water purification by efficient energy conversion. However, conventional evaporators are susceptible to fluctuations in solar radiation and the salinity of handling liquid. The present research is an innovative step toward the fabrication of superhydrophobic laser-induced graphene (LIG) interfacial evaporators for desalination and brine treatment. The fabricated dual-sided superhydrophobic laser-induced graphene (DSLIG) exhibits self-cleaning ability on both sides, enhancing salt rejection capabilities through a lotus effect. This multilayered evaporator comprises a top layer of MPES LIG and a bottom layer of PVDF AR 972 LIG, resulting in superior localized heat generation ability. The engineered surface has undergone performance analysis with DI water and NaCl solutions with concentrations of 3.5-24 wt %. The dual-stacked configuration with coupled solar (one sun)-joule heating (5 V) attained evaporation rates of ∼5 kg m