炼油厂
环境科学
石油化工
环境化学
挥发性有机化合物
分摊
环境工程
化学
政治学
有机化学
法学
作者
Birnur Buzcu,Matthew P. Fraser
标识
DOI:10.1016/j.atmosenv.2005.12.020
摘要
Hourly concentrations of ambient volatile organic compounds (VOCs) were analyzed between June and October 2003 at three sites, in order to further understand emissions of VOCs in the Houston area. Ambient concentrations of 54 VOCs from three monitoring sites in the heavily industrialized Houston Ship Channel were analyzed using positive matrix factorization (PMF). Hourly concentrations were divided into weekly data sets and analyzed to determine the most important source types that contribute to the measured VOC concentrations at these three sites. For each monitoring site, three or four sources were identified for each week as major contributors to ambient VOC concentrations using PMF. The sources isolated by the model are consistent with the chemical compositions of refinery, petrochemical and evaporative emissions, which are also the dominant inventoried sources of VOCs in Houston Ship Channel region. A night-time data analysis was also performed at two sites to investigate the effect of photochemical reactions on source attribution of VOCs.
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