Photocatalytic and Electrocatalytic Generation of Hydrogen Peroxide: Principles, Catalyst Design and Performance

催化作用 背景(考古学) 过氧化氢 试剂 过程(计算) 纳米技术 化学 计算机科学 材料科学 工艺工程 环境科学 生化工程 工程类 有机化学 古生物学 操作系统 生物
作者
Yan Guo,Xili Tong,Nianjun Yang
出处
期刊:Nano-micro Letters [Springer Nature]
卷期号:15 (1) 被引量:53
标识
DOI:10.1007/s40820-023-01052-2
摘要

Abstract Hydrogen peroxide (H 2 O 2 ) is a high-demand organic chemical reagent and has been widely used in various modern industrial applications. Currently, the prominent method for the preparation of H 2 O 2 is the anthraquinone oxidation. Unfortunately, it is not conducive to economic and sustainable development since it is a complex process and involves unfriendly environment and potential hazards. In this context, numerous approaches have been developed to synthesize H 2 O 2 . Among them, photo/electro-catalytic ones are considered as two of the most promising manners for on-site synthesis of H 2 O 2 . These alternatives are sustainable in that only water or O 2 is required. Namely, water oxidation (WOR) or oxygen reduction (ORR) reactions can be further coupled with clean and sustainable energy. For photo/electro-catalytic reactions for H 2 O 2 generation, the design of the catalysts is extremely important and has been extensively conducted with an aim to obtain ultimate catalytic performance. This article overviews the basic principles of WOR and ORR, followed by the summary of recent progresses and achievements on the design and performance of various photo/electro-catalysts for H 2 O 2 generation. The related mechanisms for these approaches are highlighted from theoretical and experimental aspects. Scientific challenges and opportunities of engineering photo/electro-catalysts for H 2 O 2 generation are also outlined and discussed.
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