Hygroscopic Nature of Lithium Ions: A Simple Key to Super Tough Atmosphere-Stable Hydrogel Electrolytes

Gel electrolytes have emerged as a versatile solution to address numerous limitations associated with liquid electrolytes in electrical energy storage (EES) devices, in terms of safety, flexibility, and affordability. Aqueous gel electrolytes, in particular, exhibit exceptional features by offering one of the highest ion solvation capacities and ionic conductivities. The two main challenges with hydrogel electrolytes are their easy freezing at subzero temperatures and rapid dehydration under open conditions, leading to the failure of the EES device. In response, we present an uncomplicated and quick-to-make hydrogel electrolyte system offering impressive mechanical properties (205.5 kPa tensile strength, 2880 kJ/m