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Dissecting Drivers of Ozone Pollution during the 2022 Multicity Lockdowns in China Sheds Light on Future Control Direction

环境科学 氮氧化物 污染 臭氧 空气污染 地面臭氧 氮氧化物 大气科学 气象学 环境工程 地理 化学 废物管理 工程类 生态学 有机化学 生物 地质学 燃烧
作者
Yue Tan,Yingnan Zhang,Tao Wang,Tianshu Chen,Jiangshan Mu,Likun Xue
出处
期刊:Environmental Science & Technology [American Chemical Society]
卷期号:58 (16): 6988-6997 被引量:14
标识
DOI:10.1021/acs.est.4c01197
摘要

In 2022, many Chinese cities experienced lockdowns and heatwaves. We analyzed ground and satellite data using machine learning to elucidate chemical and meteorological drivers of changes in O3 pollution in 27 major Chinese cities during lockdowns. We found that there was an increase in O3 concentrations in 23 out of 27 cities compared with the corresponding period in 2021. Random forest modeling indicates that emission reductions in transportation and other sectors, as well as the changes in meteorology, increased the level of O3 in most cities. In cities with over 80% transportation reductions and temperature fluctuations within −2 to 2 °C, the increases in O3 concentrations were mainly attributable to reductions in nitrogen oxide (NOx) emissions. In cities that experienced heatwaves and droughts, increases in the O3 concentrations were primarily driven by increases in temperature and volatile organic compound (VOC) emissions, and reductions in NOx concentrations from ground transport were offset by increases in emissions from coal-fired power generation. Despite 3–99% reduction in passenger volume, most cities remained VOC-limited during lockdowns. These findings demonstrate that to alleviate urban O3 pollution, it will be necessary to further reduce industrial emissions along with transportation sources and to take into account the climate penalty and the impact of heatwaves on O3 pollution.
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