环境科学
三角洲
臭氧
长江
空气质量指数
气候学
大气科学
中国
气象学
地理
地质学
工程类
航空航天工程
考古
作者
Xiaokang Chen,Zhe Jiang,Yanan Shen,Rui Li,Yunfei Fu,Jane Liu,Han Han,Hong Liao,Xugeng Cheng,Dylan B. A. Jones,H. M. Worden,Gonzalo González Abad
摘要
Abstract Observational data indicate increasing trends of surface ozone (O 3 ) in China, despite emission controls that have resulted in reductions of precursor emissions. Here, we explore the cause of this contradiction, through analysis of surface observations (2014–2019) in China and historical observation record in the United States (US, 1990–2019). Our observation‐based analysis indicates that the reductions of nitrogen oxides (NO x ) emissions led to increase of surface O 3 in North China Plain (NCP) and Yangtze River Delta (YRD) of around 8 ppb. However, NO x controls resulted in shift of O 3 chemical regimes over NCP and YRD, with turning points between NO x ‐ and volatile organic compound (VOC)‐limited regimes around 2019, while model simulations suggest transitional or NO x ‐limited regimes over the rest of China. The impacts of high fine particles (PM 2.5 ) on O 3 formation has declined because of the reduction of PM 2.5 concentrations. Stricter NO x controls can mitigate O 3 pollutions over industrialized areas in China.
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