光催化
光降解
四环素类抗生素
材料科学
纳米技术
兴奋剂
抗生素
催化作用
化学
有机化学
四环素
光电子学
生物化学
作者
X. Wang,Jinfen Niu,Lan Yang,Xingru Guo,Xiaojiao Yu,Binghua Yao
标识
DOI:10.1002/slct.202301936
摘要
Abstract Antibiotics cause negative impacts on the ecosystem and people‘s health, and it is imperative to reduce antibiotic residuum in a green and sustainable way. There has been a broad application of photocatalytic technology in the sewage treatment field. Compared with metal oxides, graphite carbon nitride, as an n‐type non‐metallic semiconducting polymer, has an applicable energy gap, simple preparation and easily accessible. Yet the g‐C 3 N 4 of simple preparation tends to have some crucial weaknesses like rapid charge carrier recombination, underutilization of the visible spectrum and incomplete mineralization, which severely confine its farther application. Element doping modification enormously improves the separation of g‐C 3 N 4 photogenic hole‐charge, which is applied to the removal of antibiotics in wastewater. The doping modification of g‐C 3 N 4 ‐based semiconductor photocatalysts and research progress in the photocatalytic degradation of various antibiotics (sulfonamides, β‐lactam, quinolones, tetracycline) in water are reviewed in this paper, and the preparation of g‐C 3 N 4 , the sorts and principles of elemental doping are investigated, with emphasis on the application of g‐C 3 N 4 towards the photocatalytic degradation of antibiotics, and the existing problems and challenges in this field are put forward.
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