High-entropy solvent design enabling a universal electrolyte with a low freezing point for low-temperature aqueous batteries

Amide additives acting as hydrogen-bonding ligands effectively break the cross-linking structures between water molecules and increase the entropy of mixed solvents, thus enabling a mixed solvent with an ultralow freezing point of -98 °C. Zinc-ion batteries using this hybrid solvent exhibit good cycling stability over a wide temperature range from -60 °C to 50 °C.