溶剂
胺气处理
解吸
热能
化学工程
压力降
吸收(声学)
化学
热的
色谱法
材料科学
有机化学
吸附
热力学
复合材料
物理
工程类
作者
Jiafei Zhang,Yu Qiao,Wanzhong Wang,R.D. Misch,Khuram Hussain,David W. Agar
标识
DOI:10.1016/j.egypro.2013.05.224
摘要
A novel CO2 capture system using thermomorphic biphasic solvent (TBS) has been studied in this work. It exhibits a thermal-induced liquid-liquid phase separation (LLPS) behaviour, which intensifies CO2 desorption at temperature of 80 °C and therefore enables using low value heat ca. 90 °C to reduce the process operating cost. To regulate the phase change behaviour, blended amine solvents were formulated for attaining a homogeneous solution in absorption and biphasic system in regeneration. Thermal and oxidative degradations were also surveyed for the selected amines and the degradation products were analysed by gas chromatography - mass spectrometry (GC-MS). A bench-scale unit with a glass column of 40 mm inner diameter and random packings of 1 m height was employed for measuring the pressure drop and liquid hold-up as well as other physicochemical properties to assess the technical feasibility of such novel system.
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