磷酸
催化作用
选择性
工作流程
位阻效应
反应性(心理学)
对映选择合成
外推法
化学
单变量
计算化学
有机化学
组合化学
多元统计
数学
计算机科学
机器学习
数据库
数学分析
医学
替代医学
病理
作者
Jordan P. Liles,Caroline Rouget-Virbel,Julie L. Hofstra Wahlman,René Rahimoff,Jennifer M. Crawford,Abby Medlin,Veronica S. O’Connor,Junqi Li,Vladislav A. Roytman,F. Dean Toste,Matthew S. Sigman
出处
期刊:Chem
[Elsevier]
日期:2023-06-01
卷期号:9 (6): 1518-1537
被引量:10
标识
DOI:10.1016/j.chempr.2023.02.020
摘要
The widespread success of BINOL-chiral phosphoric acids (CPAs) has led to the development of several high molecular weight, sterically encumbered variants. Herein, we disclose an alternative, minimalistic chiral phosphoric acid backbone incorporating only a single instance of point chirality. Data science techniques were used to select a diverse training set of catalysts, which were benchmarked against the transfer hydrogenation of an 8-aminoquinoline. Using a univariate classification algorithm and multivariate linear regression, the key catalyst features necessary for achieving high levels of selectivity were deconvoluted, revealing a simple catalyst model capable of predicting selectivity for out-of-set catalysts. This workflow enabled extrapolation to a catalyst that provided higher selectivity than both peptide-type and BINOL-type catalysts reported previously (up to 95:5 er). These techniques were then successfully applied toward two additional transforms. Taken together, these examples illustrate the power of combining rational design with data science (ab initio) to efficiently explore reactivity during catalyst development.
科研通智能强力驱动
Strongly Powered by AbleSci AI