Research progress of ABX3-type lead-free perovskites for optoelectronic applications: materials and devices

ABX试验 材料科学 铅(地质) 光电子学 纳米技术 数学 统计 地貌学 地质学
作者
Hao Wang,Chunqian Zhang,Wenqi Huang,Xiaoping Zou,Zhenyu Chen,Shengliu Sun,Lixin Zhang,Junming Li,Jin Cheng,Shixian Huang,Mingkai Gu,Xinyao Chen,Xin Guo,Ruoxia Gui,Weimin Wang
出处
期刊:Physical Chemistry Chemical Physics [Royal Society of Chemistry]
卷期号:24 (45): 27585-27605 被引量:17
标识
DOI:10.1039/d2cp02451a
摘要

In recent years, lead halide perovskite materials have attracted great interest and are widely used in solar cells and light-emitting devices due to their high photoelectronic quantum yield, high color purity, high defect tolerance, long diffusion length, high carrier mobility, and bandgap tunability. However, the application of lead halide perovskites is limited due to the presence of Pb, making lead-free perovskites an important substitute due to their same crystal structure and similar properties. Although some reports have been made on lead-free perovskite materials, there are still great challenges to realize their application due to their poor stability, easy phase transition, and low photoelectric conversion efficiency. Here, we mainly summarize the development and application of ABX3-type lead-free halide perovskite materials, especially in optoelectronic devices. The article first introduces the lattice and energy band structure, the optoelectronic properties of lead-free perovskites, including the research method of lead-free perovskites, and then analyzes the reasons for the low luminous efficiency and poor stability of lead-free perovskite materials. Second, the development history and current situation of lead-free perovskites in different optoelectronic device applications are summarized. Finally, we present the challenges and prospects for the future development of lead-free perovskites.
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