Recent advances in biodiesel production using functional carbon materials as acid/base catalysts

生物柴油 生物柴油生产 催化作用 碳纤维 基础(拓扑) 化学 材料科学 生产(经济) 制浆造纸工业 化学工程 有机化学 数学 经济 复合材料 复合数 工程类 数学分析 宏观经济学
作者
Pan Hu,Qineng Xia,Yuan Wang,Zhangfeng Shen,Hong Huang,Zhigang Ge,Xi Li,Jian He,Xiaoqiang Wang,Lifen Li,Yangang Wang
出处
期刊:Fuel Processing Technology [Elsevier]
卷期号:237: 107421-107421 被引量:55
标识
DOI:10.1016/j.fuproc.2022.107421
摘要

Biodiesel is regarded as an excellent substitute or additive to fossil diesel. Carbon materials are favorable platform to synthesize acid and/or base catalysts for transformation of renewable oil into biodiesel owing to their remarkable merits, including structural diversity, controlled surface properties, excellent stability, and no toxicity. Due to the fast-growing development of this subject matter, it is high time to summarize the recent progress. Consequently, this review systematically summarized the most up-to-date advances on the application of functionalized carbon-based catalysts for upgrading renewable oil into biodiesel, including (1) summary of the common feedstocks for producing biodiesel; (2) synthesis methods of carbonaceous materials; (3) synthesis methods and catalytic activities of various carbon-based solid acid and base catalysts; and (4) the reusability and deactivation of the catalyst. Meanwhile, effect of physicochemical properties, including acidity/basicity, hydrophilicity/hydrophobicity, and porosity of catalysts on their catalytic activity was analyzed. Finally, a brief conclusion of this review, and challenges and future perspectives towards this subject matter were also proposed. Combination of multiple outstanding properties in a carbon-based catalyst is feasible to obtain excellent catalytic performance in production of biodiesel. We believe this review will be meaningful for developing state-of-the-art carbon-based catalyst for biodiesel production. This review systematically summarized the most up-to-date advances on the application of functionalized carbon-based catalysts for upgrading various renewable oil into biodiesel. • Carbon materials are favorable platform to synthesize the catalysts for biodiesel production. • The synthetic methods of various functional carbon materials are systematically summarized. • The catalytic activities of carbon-based acid and base catalysts are critically evaluated. • Effect of physicochemical properties of the catalysts on their catalytic activity was analyzed. • Challenges and perspectives of carbon-based catalysts for biodiesel production were proposed.
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