环境科学
生物质燃烧
空气质量指数
大气科学
冬季
气候学
地理
气象学
气溶胶
地质学
作者
El. Mehdi EL. Baramoussi,Yangang Ren,Chaoyang Xue,Ibrahim Ouchen,Véronique Daële,Patrick Mercier,Christophe Chalumeau,Frédéric L.E. Fur,Patrice Colin,Abderrazak Yahyaoui,Olivier Favez,Abdelwahid Mellouki
标识
DOI:10.1016/j.scitotenv.2022.159905
摘要
Atmospheric black carbon (BC) concentration over a nearly 5 year period (mid-2017–2021) was continuously monitored over a suburban area of Orléans city (France). Annual mean atmospheric BC concentration were 0.75 ± 0.65, 0.58 ± 0.44, 0.54 ± 0.64, 0.48 ± 0.46 and 0.50 ± 0.72 μg m −3 , respectively, for the year of 2017, 2018, 2019, 2020 and 2021. Seasonal pattern was also observed with maximum concentration (0.70 ± 0.18 μg m −3 ) in winter and minimum concentration (0.38 ± 0.04 μg m −3 ) in summer. We found a different diurnal pattern between cold (winter and fall) and warm (spring and summer) seasons. Further, fossil fuel burning contributed >90 % of atmospheric BC in the summer and biomass burning had a contribution equivalent to that of the fossil fuel in the winter. Significant week days effect on BC concentrations was observed, indicating the important role of local emissions such as car exhaust in BC level at this site. The behavior of atmospheric BC level with COVID-19 lockdown was also analyzed. We found that during the lockdown in warm season (first lockdown: 27 March–10 May 2020 and third lockdown 17 March–3 May 2021) BC concentration were lower than in cold season (second lockdown: 29 October–15 December 2020), which could be mainly related to the BC emission from biomass burning for heating. This study provides a long-term BC measurement database input for air quality and climate models. The analysis of especially weekend and lockdown effect showed implications on future policymaking toward improving local and regional air quality as well. • Five-year BC measurements were conducted in a suburban area in central France. • Strong seasonal variations and weekend effects were observed. • Biomass burning contributed to more than half of winter BC. • Lockdown in cold season and warm season had reverse effect on BC concentration.
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