合成气
煤
废物管理
天然气
煤气化
整体气化联合循环
环境科学
发电
协同生产
原材料
工艺工程
电
洁净煤技术
产量(工程)
化学
氢
材料科学
工程类
功率(物理)
有机化学
物理
公共关系
电气工程
量子力学
政治学
冶金
作者
Zheng Zhang,Lin Zhu,Jianting Yu,Huiming Liu,Qiang Hao,Yue Huang
标识
DOI:10.1002/ente.202300718
摘要
The traditional coal‐gasification process has many problems, such as low yield, large loss of syngas, and large carbon emission. Herein, a novel dual‐regulation system is established. Natural gas is used as the supplemental feed to add hydrogen‐ to coal‐gasification syngas, which is the primary regulation process. Water–gas shift process with calcium looping is treated as the secondary regulation process to regulate the ratio of H 2 to CO and CO 2 subtly. The potential feasibility of the system is verified through thermodynamic perspective by Aspen Plus. Under the simulation condition, the final methanol product amount is 3485.12 kmol h −1 with 97.2% concentration and 33.47 MWe net electricity is generated. As a result, the methanol efficiency and net electricity efficiency are 60.55% and 3.22%, respectively. For investigating the effectiveness of regulation, the effects of mass ratio of natural to coal feedstock on materials and performances are discussed.
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