资源回收
流出物
污水污泥
过氧化氢
污水处理
污水污泥处理
环境科学
污水
环境友好型
废物管理
污染物
化学需氧量
降级(电信)
制浆造纸工业
化学
环境化学
环境工程
计算机科学
工程类
废水
生态学
有机化学
电信
生物
作者
Zhiyan Liang,Qingyun Yan,Huase Ou,Da‐Wei Li,Yayun Zhang,Jinlong Zhang,Lixi Zeng,Mingyang Xing
标识
DOI:10.1073/pnas.2317394121
摘要
Effectively managing sewage sludge from Fenton reactions in an eco-friendly way is vital for Fenton technology’s viability in pollution treatment. This study focuses on sewage sludge across various treatment stages, including generation, concentration, dehydration, and landfill, and employs chemical composite MoS 2 to facilitate green resource utilization of all types of sludge. MoS 2 , with exposed Mo 4+ and low-coordination sulfur, enhances iron cycling and creates an acidic microenvironment on the sludge surface. The MoS 2 -modified iron sludge exhibits outstanding (>95%) phenol and pollutant degradation in hydrogen peroxide and peroxymonosulfate-based Fenton systems, unlike unmodified sludge. This modified sludge maintains excellent Fenton activity in various water conditions and with multiple anions, allowing extended phenol degradation for over 14 d. Notably, the generated chemical oxygen demand (COD) in sludge modification process can be efficiently eliminated through the Fenton reaction, ensuring effluent COD compliance and enabling eco-friendly sewage sludge resource utilization.
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