钙钛矿(结构)
材料科学
微晶
单晶
晶界
工程物理
薄膜
Crystal(编程语言)
光电子学
光伏系统
纳米技术
光伏
结晶学
冶金
电气工程
计算机科学
化学
微观结构
物理
工程类
程序设计语言
作者
Xiao Cheng,Shuang Yang,Bingqiang Cao,Xutang Tao,Zhaolai Chen
标识
DOI:10.1002/adfm.201905021
摘要
Abstract The efficiency of perovskite solar cells has increased to a certified value of 25.2% in the past 10 years, benefiting from the superior properties of metal halide perovskite materials. Compared with the widely investigated polycrystalline thin films, single crystal perovskites without grain boundaries have better optoelectronic properties, showing great potential for photovoltaics with higher efficiency and stability. Additionally, single crystal perovskite solar cells are a fantastic model system for further investigating the working principles related to the surface and grain boundaries of perovskite materials. Unfortunately, only a handful of groups have participated in the development of single crystal perovskite solar cells; thus, the development of this area lags far behind that of its polycrystalline counterpart. Therefore, a review paper that discusses the recent developments and challenges of single crystal perovskite solar cells is urgently required to provide guidelines for this emerging field. In this progress report, the optical and electrical properties of single crystal and polycrystalline perovskite thin films are compared, followed by the recent developments in the growth of single crystal perovskite thin films and the photovoltaic applications of this material. Finally, the challenges and perspectives of single crystal perovskite solar cells are discussed in detail.
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