Multi‐Interfacial Confined Assembly of Colloidal Quantum Dots Quasisuperlattice Microcavities for High‐Resolution Full‐Color Microlaser Arrays

材料科学 激光阈值 量子点 纳米技术 光电子学 蒸发 激光器 纳米结构 光学 热力学 物理 波长
作者
Hui Li,Yuyan Zhao,Yuchen Qiu,Hanfei Gao,Ke He,Junchuan Yang,Yingjie Zhao,Guangwen OuYang,Na Ma,Wei Xiao,Zuliang Du,Lei Jiang,Yuchen Wu
出处
期刊:Advanced Materials [Wiley]
卷期号:36 (23) 被引量:1
标识
DOI:10.1002/adma.202314061
摘要

Abstract Colloidal quantum dots (CQDs) are considered a promising material for the next generation of integrated display devices due to their designable optical bandgap and low energy consumption. Owing to their dispersibility in solvents, CQD micro/nanostructures are generally fabricated by solution‐processing methods. However, the random mass transfer in liquid restricts the programmable construction in macroscopy and ordered assembly in microscopy for the integration of CQD optical structures. Herein, a multi‐interfacial confined assembly strategy is developed to fabricate CQDs programmable microstructure arrays with a quasisuperlattice configuration through controlling the dynamics of three‐phase contact lines (TPCLs). The motion of TPCLs dominates the division of liquid film for precise positioning of CQD microstructures, while pinned TPCLs control the solvent evaporation and concentration gradient to directionally drive the mass transfer and packing of CQDs. Owing to their long‐range order and adjustable structural dimensions, CQD microring arrays function as high‐quality‐factor (high‐ Q ) lasing resonant cavities with low thresholds and tunable lasing emission modes. Through the further surface treatment and liquid dynamics control, the on‐chip integration of red (R), green (G), and blue (B) multicomponent CQD microlaser arrays are demonstrated. The technique establishes a new route to fabricate large‐area, ultrahigh‐definition, and full‐color CQD laser displays.
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