Reconstructed Water Oxidation Electrocatalysts: The Impact of Surface Dynamics on Intrinsic Activities

材料科学 纳米材料基催化剂 析氧 生化工程 催化作用 纳米技术 分解水 计算机科学 工艺工程 电化学 物理化学 电极 纳米颗粒 光催化 工程类 生物化学 化学
作者
N. Clament Sagaya Selvam,Lijie Du,Bao Yu Xia,Pil J. Yoo,Bo You
出处
期刊:Advanced Functional Materials [Wiley]
卷期号:31 (12) 被引量:261
标识
DOI:10.1002/adfm.202008190
摘要

Abstract Electroreduction of small molecules such as H 2 O, CO 2 , and N 2 for producing clean fuels or valuable chemicals provides a sustainable approach to meet the increasing global energy demands and to alleviate the concern on climate change resulting from fossil fuel consumption. On the path to implement this purpose, however, several scientific hurdles remain, one of which is the low energy efficiency due to the sluggish kinetics of the paired oxygen evolution reaction (OER). In response, it is highly desirable to synthesize high‐performance and cost‐effective OER electrocatalysts. Recent advances have witnessed surface reconstruction engineering as a salient tool to significantly improve the catalytic performance of OER electrocatalysts. In this review, recent progress on the reconstructed OER electrocatalysts and future opportunities are discussed. A brief introduction of the fundamentals of OER and the experimental approaches for generating and characterizing the reconstructed active sites in OER nanocatalysts are given first, followed by an expanded discussion of recent advances on the reconstructed OER electrocatalysts with improved activities, with a particular emphasis on understanding the correlation between surface dynamics and activities. Finally, a prospect for clean future energy communities harnessing surface reconstruction‐promoted electrochemical water oxidation will be provided.
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