Synthesis of magnetic hydrochar from Fenton sludge and sewage sludge for enhanced anaerobic decolorization of azo dye AO7

无氧运动 化学 污水污泥 厌氧消化 氧化还原 降级(电信) 污水处理 资源回收 生物降解 制浆造纸工业 废物管理 废水 无机化学 甲烷 有机化学 生物 工程类 电信 生理学 计算机科学
作者
Siqi Tong,Dan Chen,Ping Mao,Xinbai Jiang,Aiwu Sun,Zhixiang Xu,Xiaodong Liu,Jinyou Shen
出处
期刊:Journal of Hazardous Materials [Elsevier]
卷期号:424: 127622-127622 被引量:19
标识
DOI:10.1016/j.jhazmat.2021.127622
摘要

A novel magnetic hydrochar synthesized from Fenton sludge (FS) and sewage sludge (SS) was employed in the anaerobic decolorization of acid orange 7 (AO7). The stable presence of Fe3O4 in magnetic hydrochar was confirmed by physicochemical characterization. The degradation efficiency of AO7 in the anaerobic system with the addition of hydrochar prepared in an optimal proportion (SS:FS=1:3, named as HC-1:3) could reach 98.55%, which was 1.91 times higher than the control system. Particularly, superior electrical conductivity, electron transport system activity and azo reductase activity of the sludge in anaerobic system with HC-1:3 were achieved. The redox of Fe(Ⅲ)/Fe(Ⅱ) in anaerobic system was realized by dissimilatory iron-reducing bacteria enriched with HC-1:3. According to the six-cycle batch experiments and 120-day continuous-flow UASB experiments, the addition of HC-1:3 into the anaerobic system facilitated the diversity of microbiological community and increased the ecological stability of anaerobic system. The possible electron transfer mechanism involving in the magnetic hydrochar-based anaerobic system for AO7 removal was speculated preliminarily. The as-prepared magnetic hydrochar not only showed a promising future in anaerobic system for recalcitrant contaminants degradation, but also provided a new approach for the resource utilization of FS and SS.
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