Comment on “Transport of substantial stratospheric ozone to the surface by a dying typhoon and shallow convection” by Chen et al. (2022)

台风 对流层 平流层 大气科学 臭氧 环境科学 气象学 中国科学院 优势(遗传学) 中国 气候学 化学 地质学 物理 地理 考古 生物化学 基因
作者
Xiaodong Zheng,Wen Yang,Yuting Sun,Chunmei Geng,Yingying Liu,Xiaobin Xu
标识
DOI:10.5194/egusphere-2023-2336
摘要

Abstract. Chen et al. (2022) analyzed the event of rapid nocturnal O3 enhancement (NOE) observed on 31 July 2021 at surface level in the North China Plain and proposed transport of substantial stratosphere ozone to the surface by Typhoon In-fa followed by downdraft of shallow convection as the mechanism of the NOE event. The analysis seems to be valid in the view-point of atmospheric physics. This comment revisits the NOE phenomenon on the basis of the China National Environmental Monitoring Center (CNEMC) network data ever used in Chen et al. (2022), together with the CNEMC data from Zibo (ZB), and O3, NOx, PAN and VOCs data from the Zibo supersite operated by China Research Academy of Environmental Sciences (CRAES). We found (a) Ox (O3+NO2) levels during the NOE period approaching to those of O3 during 14:00–17:00 LT; (b) the relationship between O3 and PAN (peroxyacetic nitric anhydride) consistent with dominance of chemical and physical processes within the boundary layer, and (c) estimated photochemical ages of air mass being shorter than one day and showing no drastic increases during the NOE. We argue that the NOE was not caused by typhoon-induced stratospheric intrusion but originated from fresh photochemical production in the lower troposphere.

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