材料科学
兴奋剂
红外线的
发射率
分析化学(期刊)
陶瓷
杂质
光学
光电子学
物理
化学
复合材料
量子力学
色谱法
作者
Jiaqi Li,Jianyu Li,Bin Xu,Zhiyi Ren,S.L. Yan,D. Y. Zhang,Meng Wang,Xiaoliang Sun,Chi Liu,Jing Feng
标识
DOI:10.1142/s0217984924503913
摘要
This work aims to investigate the influence of Ca[Formula: see text] doping on the infrared emission properties of DyTa 3 O 9 ceramics. DyTa 3 O 9 is considered a promising high-temperature thermal protection material due to its low thermal conductivity and good high-temperature stability. However, there is currently no research on the infrared radiation performance of such materials. We synthesized DyTa 3 O 9 ceramics with different Ca[Formula: see text] doping concentrations using the solid-phase reaction method and systematically investigated the effect of doping concentration on the infrared emissivity of DyTa 3 O 9 ceramics. When Ca[Formula: see text] is doped into the DyTa 3 O 9 lattice, the original Dy elements are replaced by Ca, resulting in an increase in lattice constants and enhanced lattice distortion. The doping of Ca[Formula: see text] introduces impurity energy levels, making it possible for some low-energy electron transitions, achieving an enhancement in infrared absorption and emission capabilities. When the Ca[Formula: see text] doping concentration reaches 7.5% mol, the average infrared emissivity in the 3–5[Formula: see text][Formula: see text]m and 8–12[Formula: see text][Formula: see text]m ranges are 0.85 and 0.92, respectively, representing a 19.7% and 21% increase compared to DyTa 3 O 9 . This novel high-infrared-emissivity ceramic holds great potential for applications in high-temperature energy conservation and aerospace thermal protection.
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