光催化
纳米复合材料
辐照
可见光谱
4-硝基苯酚
光化学
材料科学
还原(数学)
纳米颗粒
化学
纳米技术
光电子学
催化作用
有机化学
物理
几何学
数学
核物理学
作者
S Al-Fakeh Maged,Ola M. El‐Borady,Hamza El-Hosainy,Maged El‐Kemary
标识
DOI:10.1007/s11356-023-30010-z
摘要
Recently, low-cost graphitic carbon nitride (g-C3N4) revealed high photocatalytic activities and provided solutions to environmental pollution. In this study, we synthesized brown mesoporous 2D g-C3N4 by calcination dicyandiamide with pluronic P123. This is followed by loading of Ag NPs on the prepared 2D g-C3N4 by photodeposition process. After that, a ternary composite 2% Ag/ 2D g-C3N4 / g-C3N4 QDs heterojunction photocatalyst has been successfully prepared. The prepared nanomaterials were comprehensively characterized by various analysis techniques such as XRD, UV-Vis., BET, XPS, SEM, TEM. This new system exhibited a large surface area with porous structure and a wide absorption of visible light. The results verified that Ag NPs decoration enhanced the charge separation of photo-generated carriers of g-C3N4 2D and g-C3N4 QDs, promote significant enhancement in the photocatalytic activity for reduction of p-nitrophenol with a rate constant (k) value of 0.49729 / min in 6 min. This rate is about two-fold higher than that observed for pure g-C3N4 2D and g-C3N4 QDs as well as shows an improvement compared to 2% Ag/ g-C3N4 2D and g-C3N4 2D/ g-C3N4 QDs. The results open the door to design highly efficient 2D/0D nanocomposite photocatalysts for a wide variety of environmental applications.
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