多金属氧酸盐
催化作用
范围(计算机科学)
纳米技术
材料科学
分解水
领域(数学)
功能(生物学)
化学
计算机科学
有机化学
光催化
生物
进化生物学
数学
程序设计语言
纯数学
作者
Rongji Liu,Carsten Streb
标识
DOI:10.1002/aenm.202101120
摘要
Abstract Single atom catalysts—SACs—have received intense interest in sustainable energy research due to their enormous application potential and broad catalytic scope. In particular, SACs anchored on molecular metal oxides—polyoxometalates (POMs)—offer unrivalled possibilities as models to understand the function of these complex systems on the atomic level. Research questions which are difficult to address for classical heterogeneous SACs can be addressed by experiment and theory using POM‐SACs as prototype catalysts. This review reviews the emerging field of POM‐SAC research with a focus on fundamental properties and their application in energy conversion and storage technologies including water splitting, CO/CO 2 ‐ as well as N 2 ‐activation. Current limitations of the field are identified and possible routes to overcome these are described. Future areas of development, including polyoxometalate‐single‐site catalysts, are highlighted, and critically assessed to enable the community to develop this fast‐moving field further.
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