异质结
材料科学
钙钛矿(结构)
平面的
图层(电子)
金属
光电子学
曲面(拓扑)
复合材料
化学
计算机科学
结晶学
冶金
计算机图形学(图像)
几何学
数学
作者
Lin Yang,Chunxiang Dall’Agnese,Yohan Dall’Agnese,Gang Chen,Yu Gao,Yoshitaka Sanehira,Ajay Kumar Jena,Xiaofeng Wang,Yury Gogotsi,Tsutomu Miyasaka
标识
DOI:10.1201/9781003306511-50
摘要
MXenes are a large and rapidly expanding family of 2D materials that, owing to their unique optoelectronic properties and tunable surface termination, find a wide range of applications including energy storage and energy conversion. In this work, Ti3C2Tx MXene nanosheets are applied as a novel type of electron transport layer (ETL) in low-temperature processed planarstructured perovskite solar cells (PSCs). Interestingly, simple UV-ozone treatment of the metallic Ti3C2Tx that increases the surface Ti–O bonds without any change in its bulk properties such as high electron mobility improves its suitability as an ETL. Improved electron transfer and suppressed recombination at the ETL/perovskite interface results in augmentation of the power conversion efficiency (PCE) from 5.00% in the case of Ti3C2Tx without UV-ozone treatment to the champion PCE of 17.17%, achieved using the Ti3C2Tx film after 30 min of UV-ozone treatment.
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