激子
等离子体子
散射
纳米光子学
吸收(声学)
分子物理学
吸收光谱法
物理
超短脉冲
原子物理学
光电子学
凝聚态物理
光学
激光器
作者
Rongguang Du,Huatian Hu,Tong Fu,Zhifeng Shi,Shunping Zhang,Hongxing Xu
出处
期刊:Nano Letters
[American Chemical Society]
日期:2023-01-03
卷期号:23 (2): 444-450
被引量:11
标识
DOI:10.1021/acs.nanolett.2c03385
摘要
We unambiguously extract the individual decay channels of a coupled plasmon-exciton system by using correlated single-particle absorption and scattering measurements. A remarkable difference in the two channels is present─clear Rabi splitting in the plasmon channel but no Rabi splitting in the exciton channel. Discordance in the absorption and scattering spectra are mainly originated from the distinct contributions of plasmon and exciton channels in the absorption and scattering process. Our findings provide insights into plasmon-exciton interaction in an open cavity and can impact the design of plexcitonic devices for ultrafast nonlinear nanophotonics.
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